Magnetic anisotropy and spin polarizability are recognized as the critical parameters determining the performance of ferromagnetic electrodes in spintronic devices. Fe
4N exhibits a high Curie temperature, high saturation magnetization, and good stability; however, the application in spintronic devices is limited by the low spin polarizability and in-plane magnetic anisotropy (IMA). Atomic doping is an effective method to modulate the magnetic properties of Fe
4N. As a heavy metal element, Pt exhibits a strong spin-orbit coupling (SOC) effect. Doping Pt into Fe
4N effectively enhances the overall SOC strength of the system, thereby realizing the regulation of the electronic structure and magnetic properties of the material. In this work, the electronic structure and magnetic properties of Pt
cFe
3N were investigated based on the first - principles calculations. The calculated results show that Pt
cFe
3N maintains a cubic anti-perovskite structure with a lattice constant of 3.856 Å. Phonon spectrum and ab initio molecular dynamics simulations confirm that Pt
cFe
3N possesses excellent dynamic and thermodynamic stability. The band structure calculations reveal that Pt
cFe
3N exhibits metallic properties. The band structure of Pt
cFe
3N shows no significant change upon the inclusion of SOC. The band distribution trends along all high-symmetry paths in the Brillouin zone are nearly identical whether SOC is considered or not. The total magnetic moment of Pt
cFe
3N is 8.18
μB without considering SOC. The atomic magnetic moments of FeII and Pt are 2.58
μB and 0.42
μB, respectively. The total magnetic moment of Pt
cFe
3N increases from 8.18 to 8.47
μB when SOC is considered, which is primarily due to the SOC-induced orbital contributions of 0.06
μB and 0.14
μB from the FeII and Pt atoms, respectively. The strong SOC associated with Pt atoms effectively lifts the d-orbital degeneracy and induces an orbital magnetic moment, which in turn enhances the total magnetic moment of the system. The spin polarizability of Pt
cFe
3N is -70.4%, which is 1.47 times larger than that of Fe
4N (- 47.9%). In addition, the incorporation of Pt atoms induces the transformation of Fe
4N from a weak IMA of 0.029 J/cm
3 to a weak perpendicular magnetic anisotropy (PMA) of -0.003 J/cm
3. The contributions of FeIIAa (5.104 J/cm
3) and FeIIB (- 5.104 J/cm
3) atoms to the MCA cancel each other in the system, and the Pt atom contributes an MCA of - 0.003 J/cm
3, leading to a weak PMA in Pt
cFe
3N. In summary, Pt
cFe
3N exhibits a large magnetic moment, high spin polarizability, and weak PMA, demonstrating significant application potential in the field of next-generation spintronic devices.