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中国物理学会期刊

利用多个带孔镜高效产生和分离高重频高次谐波

Efficient generation and separation of high-repetition-rate high-order harmonics by multiple drilled mirrors

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  • 飞秒激光与惰性气体相互作用产生高次谐波是目前获得阿秒激光的重要手段,同时高次谐波波段覆盖极紫外到X射线,具有相干时间分辨特性,是时间分辨角分辨光电子能谱、瞬态吸收光谱、相干衍射成像等研究的重要光源。本文基于中心波长1030 nm、重复频率500 kHz、平均功率208 W、脉冲宽度170 fs的Yb光纤飞秒激光器,驱动氩气产生光子能量覆盖27~47 eV的高次谐波。实验中利用多个带孔镜将高斯型驱动光束转换为环形贝塞尔光束,产生高次谐波并将其与驱动激光有效分离,测量结果显示该方法对驱动激光的衰减比达到10-3量级,而对高次谐波无损传输。同时理论上模拟了驱动激光经过多个带孔镜后的光斑演化及功率变化,证明这是实现高重频高平均功率飞秒激光驱动高次谐波产生并高效分离的有效手段,对于时间分辨泵浦-探测实验尤其适用。

    Based on high-order harmonic generation (HHG), coherent light sources spanning from the extreme ultraviolet to X-ray regions can be obtained, which can be applied in research such as time- and angle-resolved photoemission spectroscopy (Tr-ARPES), attosecond transient absorption spectroscopy (ATAS), and coherent diffraction imaging (CDI). As the repetition rate and power of HHG driving lasers continue to increase, effectively separating the generated high-order harmonics from the high-power driving laser has become a critical challenge. Typically, components such as grazing incidence plates (GIP), diffraction gratings, microchannel plates (MCP), and drilled mirrors (DM) are used to attenuate the high-power driving laser. However, some of these components lead to substantial loss of high-order harmonic power, or lack sufficient flexibility in optical path design.
    This paper presents a method for efficient generation and separation of high-order harmonics using multiple drilled mirrors. The setup includes four drilled mirrors (DM1–DM4), one focusing mirror, one gas jet, and one metal filter. DM1 splits the incident high-power driving laser; DM2 generates an annular driving laser; and DM3 and DM4 are used to separate the residual driving laser. In addition, DM2 and DM3 are positioned at the object plane and image plane of the focusing mirror, respectively.
    To validate the proposed method, we utilized a Yb fiber femtosecond laser (central wavelength: 1030 nm, repetition rate: 500 kHz, average power: 208 W, pulse duration: 170 fs) to drive argon gas, generating high-order harmonics with photon energies spanning 27–47 eV. The experimental results demonstrate that the method achieves an attenuation ratio of the driving laser on the order of 10-3, while enabling nearly lossless transmission of the high-order harmonics. Furthermore, theoretical simulations of the beam profile evolution and power variation during laser propagation confirm the effectiveness of this approach for high-repetition-rate, high-average-power femtosecond laser-driven HHG and efficient harmonic separation. The method is particularly suitable for time-resolved pump–probe experiments and is expected to play a significant role in the future development of large-scale attosecond laser facilities.

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