搜索

x
中国物理学会期刊

X射线发射谱方法学及中能发射谱仪技术进展

Methodology of X-ray Emission Spectroscopy and Technical Developments of Tender X-ray Emission Spectrometers

PDF
导出引用
  • X射线发射谱(XES)凭借其高能量分辨探测能力,以及对材料占据态电子结构的敏感性,成为揭示材料化学价态、配位环境及电子相互作用的核心分析手段,在量子材料、能源催化、生命科学等领域具有不可替代的价值。本文首先简要介绍了基于常规实验室及同步辐射XES谱仪技术,尤其是共振非弹性X射线散射(RIXS)谱仪的发展及应用。进而,结合中能XES广泛的应用背景,阐明了中能XES谱仪的设计原理、几种几何构型以及优缺点,系统梳理了近二十年基于实验室源和同步辐射源的中能XES谱仪技术进展,并重点关注适用于原位实验谱仪的研发与应用实例。最后,探讨了中能XES谱仪在技术应用中面临的挑战与未来发展方向,并对中能原位XES方法学的技术路线提出了思考。本文重点总结了中能XES装置的最新进展及相关应用,旨在帮助研究者深入理解该技术,拓展其应用领域,并为后续中能XES装置的研发与优化提供基础参考。

    X-ray emission spectroscopy (XES) is a non-destructive photon-in/photon-out technique that provides exceptional chemical sensitivity to the occupied electronic states of materials. It enables quantitative insights into oxidation states, coordination environments, charge-transfer interactions, and spin states, and has emerged as an indispensable probe for electronic structure characterization across diverse fields, including quantum materials, energy catalysis, and life sciences. With the continuous development of laboratory X-ray sources, synchrotron radiation facilities, and X-ray free-electron lasers, XES methodologies have been progressively refined, evolving toward higher energy resolution and enhanced sensitivity. This review first introduces the fundamental principles of both non-resonant and resonant XES, as well as the categories of electronic structure information that can be extracted from these techniques. It then outlines the development and implementation of laboratory-based and synchrotron-based XES spectrometers, with particular emphasis on resonant inelastic X-ray scattering (RIXS) instrumentation and its applications. At present, both hard and soft X-ray emission spectroscopy have become technologically mature platforms worldwide. In contrast, XES operating in the tender X-ray energy regime(2000—5000 eV) has progressed more slowly due to the special photon energy range, limitations in crystal optics, and the relatively limited availability of synchrotron beamlines in this regime. Meanwhile, the tender X-ray energy range encompasses light elements such as P, S, and Cl, as well as 4d transition metals, which play pivotal roles in catalysis, energy conversion, and biological systems. Accurate characterization of their electronic structures is therefore essential for advancing research in these areas. Motivated by these scientific demands, this review systematically discusses the design principles and geometrical configurations of tender XES spectrometers, analyzes their respective advantages and limitations, and compares different configurations in terms of energy resolution, diffraction efficiency, energy coverage, and experimental compatibility. Furthermore, we comprehensively summarize the technical progress achieved over the past two decades in tender XES instrumentation based on both laboratory and synchrotron radiation sources. This review aims to provide researchers with a deeper understanding of the tender XES methodology and its potential extensions to broader applications, while also laying a foundation for the development and optimization of future XES instrumentation in this energy regime.
    In addition, catalytic reactions, biological processes, and electrochemical battery systems typically occur under dynamic conditions, often involving liquid phases, multiphase interfaces, and complex reaction pathways. Considering these characteristics, this review places particular emphasis on the compatibility of tender XES spectrometers with sample environments under in situ/operando conditions. We discuss the development and application of tender XES in situ/operando infrastructure, including helium gloveboxes, dedicated sample chambers, and gas reaction cells. Finally, we examine the remaining technical challenges associated with practical applications of tender XES and outline future developmental directions, together with our perspective on methodological strategies for enabling operando XES in this energy regime.

    目录

    返回文章
    返回
    Baidu
    map