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Abstract

One-dimensional (1D) graphene superlattices were formed on a prototypical high index surface-Cu(410)-O. Atomic hydrogen adsorption on the superlattice was studied by using Raman spectroscopy, low-energy electron diffraction (LEED) and scanning tunneling microscopy (STM). Selective H adsorption due to the 1D modulation from the Cu substrate was observed in defect-free graphene area. Most H adatoms occupy the same positions in the 1D graphene superlattice stripes, as revealed by STM. This opens the possibility for further graphene property tuning through 1D superlattices. In addition to H monomers and dimers, a new type of trimer configuration was also observed.

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Funds:Project supported by the National Basic Research Program of China (Grant No. 2012CB921300), and the National Natural Science Foundation of China (Grant Nos. 11074005, 91021007).

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Vol. 63, Issue 19 - 2014-10-05

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