LUO Santu; ZHANG Mingyan; ZHANG Jishen; WANG Zifeng; SUN Bowen; LIU Dingxin; RONG Mingzhe

doi:10.7498/aps.74.20251221

Abstract

Atmospheric-pressure low-temperature plasma has been widely used in various fields such as biomedicine, environmental protection, and nanomanufacturing, and the key physicochemical processes in these applications involve the interactions between plasma and aqueous solutions. However, such plasma-liquid interactions are very complex, involving a wide range of gas-liquid phase reactions as well as coupled mass transfer processes. These intricate mechanisms make it challenging for existing experimental techniques to provide a systematic understanding, thereby highlighting the critical role of simulation studies. Over the past decade, significant progress has been made in the simulation of plasma-solution interactions. Researchers have basically solved the problems of scarce transport and reaction parameter data, established various types of simulation models, and actively explored new simulation methods based on intelligence algorithms. These advances have greatly deepened our understanding of this field. Thus, this paper reviews recent developments in simulation studies of plasma-solution interactions from three perspectives, namely parameter acquisition, model construction, and intelligent algorithms, with the aim of providing useful insights for researchers.

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Corresponding author: LIU Dingxin, liudingxin@mail.xjtu.edu.cn

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Cited By

DownLoad: Full-Size Img PowerPoint

粒子类别	示例粒子	常用检测手段	主要挑战/局限性
长寿命粒子	H₂O₂, O₃, NO, N₂O₅	分光光度法; 光化学荧光探针法	非特异性, 受其他粒子干扰; 需要特定pH条件; 试剂难溶于水
短寿命粒子	¹O₂, O, OH	电子自旋共振谱法; 光化学荧光探针法	非特异性, 受其他粒子干扰; 需要特定pH条件; 捕捉剂昂贵且易被氧化
激发态分子/离子	N₂(v), ONOO^–	发射光谱法; 液相色谱法	灵敏度低; 粒子猝灭快, 难以原位检测; 温度敏感

DownLoad: CSV

工作气体	$ \sigma $/Å	ε/K	工作气体	$ \sigma $/Å	ε/K
N₂	3.56	102	CO₂	3.76	244
O₂	3.44	125	He	2.57	10.2
Ar	3.43	122	Air	3.71	78.5

DownLoad: CSV

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Vol. 74, Issue 23 - 2025-12-05

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